Thursday, 12 April 2012

Chelator Enhances Biocide Efficacy in Inhibiting SRB Biofilm Growth


A review of: Wen J, Zhao K, Gu T, Raad II (2009) A green biocide enhancer for treatment of sulphate-reducing bacteria (SRB) biofilms on carbon steel surfaces using glutaraldehyde. International Biodeterioration & Biodegradation, 63: 1102-11106.

Bacterial biofilms cause various problems such as fouling of water cooling systems, medical infections, product contamination and microbiologically influenced corrosion (MIC). MIC is responsible for billions of dollars in losses each year for many industries and account for as much as 20% of all forms of corrosion, mostly caused by sulphate reducing bacteria (SRB). Ethylenediaminetetraacetic acid (EDTA) is a chelating agent and is widely used to eradicate biofilms on catheters when combined with antibiotics. Previous experiments have also shown that EDTA combined with glutaraldehyde and tetrakis hydroxymethyl phosphonium sulphate (THPS) can enhance the inhibition of planktonic SRB growth. However, EDTA is not very biodegradable and so a search for a more environmentally friendly chelator to replace EDTA has been the impetus for the investigation by Wen et al (2009).

Ethylenediaminedisuccinate (EDDS) and glutaraldehyde were chosen for the experiment because EDDS is a popular biodegradable chelating agent and glutaraldehyde is a widely used broad spectrum biocide. SRB Desulfovibrio desulfuricans subsp. aestuarii ATCC 14563 were grown to approximately 4.3-5.1 x 105 cells ml-1 before being placed in anaerobic vials containing different concentration of EDDS and glutaraldehyde, and carbon steel coupons on which the biofilms would grow. The coupons were observed using a SEM after eight days to determine whether SRB biofilm formation was inhibited. The same experiment was conducted using pre-existing SRB biofilms to determine the efficacy of EDDS and glutaraldehyde in treating established biofilms. In addition, the effect of the biocide enhancer and the biocide was also tested on the growth of planktonic forms of the bacteria, enumerated using a haemocytometer and a light microscope.

Glutaraldehyde was shown to inhibit or delay SRB proliferation after 8 days, with 30 ppm of glutaraldehyde combined with 2000 ppm of EDDS found to be highly effective in inhibiting planktonic and sessile bacterial growth, as well as preventing biofilm formation on the coupons. Biofilms protect bacteria from biocides like glutaraldehyde therefore its use in conjunction with EDDS is far more effective than a higher concentration of glutaraldehyde or EDDS alone. Trace metals are necessary for bacterial metabolism and biofilm formation. Using chelating agents like EDDS sequester trace metals, thus limiting bacterial adhesion and growth. Chelators can also remove divalent cations from lipopolysaccharide, resulting in increased permeability of bacterial cells. EDDS enhances the biocide activity of glutaraldehyde by making it easier for glutaraldehyde to penetrate SRB biofilms and the membranes of bacteria. Because the experiment used a relatively high concentration of EDDS, a progression from the existing study would be to find an optimal balance between chelator and biocide concentration for various industrial applications.              

2 comments:

Corin Liddle said...

Interesting, could such compounds be used to prevent Accelerated Low Water Corrosion?

Mario Lewis said...

Hey Corin,

I don't see why not. We had some experience using glutaraldehyde in electron microscopy and what it does is it cross links proteins in a cell because of terminal aldehyde groups. That must be the same process in its biocide activity. I do recall having to fill in COSHH forms because glutaraldehyde is quite harmful. I dont know what the implications of regular long term glutaraldehyde treatment but I'm sure the biodegradability of EDDS may be a suited for regular applications to prevent or limit biofilm formation by chelating metal ions necessary for bacterial growth.